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Intensification of ozonation processes in a novel, compact, multi-orifice oscillatory baffled column

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journal contribution
posted on 13.06.2016, 14:57 by Marco S. Lucas, Nuno Reis, Gianluca Li-Puma
A novel approach for the intensification of ozonation of water and wastewater is presented using a highly efficient and compact Multi-Orifice Oscillatory Baffled Column (MOBC) ozonation contactor. The MOBC uniquely yielded full (i.e. 100%) use of the ozone supplied with a very short (2.25 min) liquid contact time under continuous operation and reducing the need of further gas-liquid contacting equipment downstream from the MOBC. The increased performance of the MOBC ozonation reactor was benchmarked against a bubble column (BC) design and resulted in 20% increase on the rate of p-hydroxybenzoic acid (p-HBA) degradation, 75% increase in the rate of mineralization of p-HBA per mole of ozone consumed, and 3.2-fold increase in the rate of mineralization of p-HBA per mole of ozone supplied. This results from the very small size of bubbles (few hundreds of microns) and enhanced gas-liquid mass transfer and hold-up generated in the presence of small fluid pulsations and orifice baffles.

Funding

This paper was funded by the Enterprise Office and the Enterprise Project Group of Loughborough University for funding the EPSRC Impact Acceleration Account project (EPG55-P4, EPG64-P2).

History

School

  • Aeronautical, Automotive, Chemical and Materials Engineering

Department

  • Chemical Engineering

Published in

CHEMICAL ENGINEERING JOURNAL

Volume

296

Pages

335 - 339 (5)

Citation

LUCAS, M.S., REIS, N.M. and LI PUMA, G., 2016. Intensification of ozonation processes in a novel, compact, multi-orifice oscillatory baffled column. Chemical Engineering Journal, 296, pp. 335-339.

Publisher

© Elsevier

Version

AM (Accepted Manuscript)

Publisher statement

This work is made available according to the conditions of the Creative Commons Attribution-NonCommercial-NoDerivatives 4.0 International (CC BY-NC-ND 4.0) licence. Full details of this licence are available at: https://creativecommons.org/licenses/by-nc-nd/4.0/

Publication date

2016

Notes

This paper was accepted for publication in the journal Chemical Engineering Journal and the definitive published version is available at http://dx.doi.org/10.1016/j.cej.2016.03.050.

ISSN

1385-8947

Language

en

Exports