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Which wavenumbers determine the thermodynamic stability of soft matter quasicrystals?

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journal contribution
posted on 2019-08-29, 08:58 authored by Daniel Ratliff, Andrew ArcherAndrew Archer, P Subramanian, AM Rucklidge
For soft matter to form quasicrystals an important ingredient is to have two characteristic lengthscales in the interparticle interactions. To be more precise, for stable quasicrystals, periodic modulations of the local density distribution with two particular wavenumbers should be favored, and the ratio of these wavenumbers should be close to certain special values. So, for simple models, the answer to the title question is that only these two ingredients are needed. However, for more realistic models, where in principle all wavenumbers can be involved, other wavenumbers are also important, specifically those of the second and higher reciprocal lattice vectors. We identify features in the particle pair interaction potentials which can suppress or encourage density modes with wavenumbers associated with one of the regular crystalline orderings that compete with quasicrystals, enabling either the enhancement or suppression of quasicrystals in a generic class of systems.

Funding

L’Oréal UK and Ireland Fellowship for Women in Science

Leverhulme Trust (RF-2018-449/9

Quasicrystals: how and why do they form?

Engineering and Physical Sciences Research Council

Find out more...

Quasicrystals: how and why do they form?

Engineering and Physical Sciences Research Council

Find out more...

History

School

  • Science

Department

  • Mathematical Sciences

Published in

Physical Review Letters

Volume

123

Issue

14

Publisher

American Physical Society

Version

  • AM (Accepted Manuscript)

Rights holder

© American Physical Society

Publisher statement

This paper was accepted for publication in the journal Physical Review Letters and the definitive published version is available at https://doi.org/10.1103/PhysRevLett.123.148004.

Acceptance date

2019-08-28

Publication date

2019-10-01

Copyright date

2019

ISSN

0031-9007

eISSN

1079-7114

Language

  • en

Depositor

Prof Andrew Archer

Article number

148004

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