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Supplementary information files for "On the engineering of higher-order Van Hove singularities in two dimensions"

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posted on 2025-04-29, 13:52 authored by Anirudh ChandrasekaranAnirudh Chandrasekaran, Luke C Rhodes, Edgar Abarca Morales, Carolina A Marques, Phil DC King, Peter Wahl, Joseph BetourasJoseph Betouras

Supplementary files for article "On the engineering of higher-order Van Hove singularities in two dimensions"

The properties of correlated electron materials are often intricately linked to Van Hove singularities (VHS) in the vicinity of the Fermi energy. The class of these VHS is of great importance, with higher-order ones—with power-law divergence in the density of states—leaving frequently distinct signatures in physical properties. We use a new theoretical method to detect and analyse higher-order VHS (HOVHS) in two-dimensional materials and apply it to the electronic structure of the surface layer of Sr2RuO4. We then constrain a low energy model of the VHS of the surface layer of Sr2RuO4 against angle-resolved photoemission spectroscopy and quasiparticle interference data to analyse the VHS near the Fermi level. We show how these VHS can be engineered into HOVHS.

©The Author(s), CC BY-4.0

Funding

Designing and exploring new quantum materials based on Fermi surface topological transitions

Engineering and Physical Sciences Research Council

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Strain-tuning electronic structure and quantum many-body interactions

Engineering and Physical Sciences Research Council

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Controlling Emergent Orders in Quantum Materials

Engineering and Physical Sciences Research Council

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Strain-Tuning of Emergent states of Matter

Engineering and Physical Sciences Research Council

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The Leverhulme Trust RPG-2022-315

Swiss Government Excellence Scholarship (ESKAS No. 2023.0017)

EPCC Tier 2 HPC Service

Engineering and Physical Sciences Research Council

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