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Layer-dependent properties of material extruded biodegradable polylactic acid

journal contribution
posted on 27.01.2020 by Alper Ekinci, Andrew Johnson, Andy Gleadall, Daniel Engstrom, Xiaoxiao Han
Polylactic acid (PLA) is a biodegradable, biocompatible and non-toxic biopolymer with good mechanical properties, and is commonly used for the additive manufacture of PLA-based biomedical devices. Such devices are available in a range of sizes and thicknesses, with smaller devices capable of being realised via additive manufacturing in just a few layers. Due to their thermal history and thermal degradation, the thermal, molecular weight and mechanical properties of each layer was different when the raw material was melted, and the in-course layer was deposited to the previous layer. This study investigated the effect of the number of layers on mechanical, thermal and molecular weight properties, and the relationship between them. Material extruded ISO 527–2 type 5A specimens with 1-, 2-, 3-, 4-, 5-, 7- and 10-layers were prepared with the cutting die. Results indicated that the degree of crystallinity was found to decrease from 8% to 0.5% with an increasing number of layers. This was likely due to different cooling rates, where the molecular weight was lowest for 1-layer and increased with the increasing number of layers until it almost reached that of the bulk material. Additionally, ultimate tensile strength and strain increased with an increasing number of layers, while Young's Modulus decreased due to heterogeneous material structure. Of all obtained results, there was no significant difference between 5- and 10-layer in terms of mechanical and thermal properties.

Funding

Ministry of National Education (Republic of Turkey)

Huxiang High-level Talent Gathering Project (No. 2019RS1019) from China Hunan Provincial Science and Technology Department

History

School

  • Design
  • Mechanical, Electrical and Manufacturing Engineering

Published in

Journal of the Mechanical Behavior of Biomedical Materials

Volume

104

Publisher

Elsevier

Version

AM (Accepted Manuscript)

Rights holder

© Elsevier Ltd

Publisher statement

This paper was accepted for publication in the journal Journal of the Mechanical Behavior of Biomedical Materials and the definitive published version is available at https://doi.org/10.1016/j.jmbbm.2020.103654.

Acceptance date

23/01/2020

Publication date

2020-01-25

Copyright date

2020

ISSN

1751-6161

Language

en

Depositor

Dr Andrew Johnson. Deposit date: 24 January 2020

Article number

103654

Exports