Here we present the verification of shear-mediated contributions to multiple scattering of ultrasound in suspensions. Acoustic spectroscopy was carried out with suspensions of silica of differing particle sizes and concentrations in water to find the attenuation at a broad range of frequencies. As the particle sizes approach the nanoscale, commonly used multiple scattering models fail to match experimental results. We develop a new model, taking into account shear mediated contributions, and find excellent agreement with the attenuation spectra obtained using two types of spectrometer. The results determine that shear-wave phenomena must be considered in ultrasound characterisation of nanofluids at even relatively low concentrations of scatterers that are smaller than one micrometre in diameter.
Funding
The authors acknowledge funding from the EPSRC,
grant number EP/L018780/1
History
School
Aeronautical, Automotive, Chemical and Materials Engineering
Department
Chemical Engineering
Published in
Nanoscale
Volume
8
Issue
10
Pages
5497 - 5506
Citation
FORRESTER, D.M. ...et al., 2016. Experimental verification of nanofluid shear-wave reconversion in ultrasonic fields. Nanoscale, 8 (10), pp. 5497-5506.
This work is made available according to the conditions of the Creative Commons Attribution 3.0 Unported (CC BY 3.0) licence. Full details of this licence are available at: http://creativecommons.org/licenses/by/3.0/
Acceptance date
2015-12-30
Publication date
2015-12-31
Notes
This is an Open Access Article. It is published by Royal Society of Chemistry under the Creative Commons Attribution 3.0 Unported Licence (CC BY). Full details of this licence are available at: http://creativecommons.org/licenses/by/3.0/. The dataset which supports this article can be found at http://dx.doi.org/10.17028/rd.lboro.2056149